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Multiple Meanings
harmonious — as in:  live together harmoniously

We work to encourage the harmonious coexistence of different cultures.
co-existing peacefully; or having components that are combined in a pleasing way
harmonious — as in:  soothing, harmonious music

The changes created a more harmonious melody.
pleasing — especially of music or sound

Harmony in the expression, live together in harmony, is just another form of this word. However, in the expression, the harmony of the music, it refers technically to the structure of the music. In that instance, it is neutral with regard to how good the music sounds, or how well the pieces fit together.
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